Phonon-induced decoherence and dissipation in donor-based charge qubits

We investigate the phonon-induced decoherence and dissipation in a donor-based charge quantum bit realized by the orbital states of an electron shared by two dopant ions which are implanted in a silicon host crystal. The dopant ions are taken from the group-V elements Bi, As, P, Sb. The excess electron is coupled to deformation potential acoustic phonons which dominate in the Si host. The particular geometry tailors a non-monotonous frequency distribution of the phonon modes. We determine the exact qubit dynamics under the influence of the phonons by employing the numerically exact quasi-adiabatic propagator path integral scheme thereby taking into account all bath-induced correlations. In particular, we have improved the scheme by completely eliminating the Trotter discretization error by a Hirsch-Fye extrapolation. By comparing the exact results to those of a Born-Markov approximation we find that the latter yields appropriate estimates for the decoherence and relaxation rates. However, noticeable quantitative corrections due to non-Markovian contributions appear.Comment: 8 pages, 8 figures, published online in Eur.Phys.J.B, article in press; the original publication is avaiable at www.eurphysj.or

Dynamical bistability in the driven circuit QED

We show that the nonlinear response of a driven circuit quantum electrodynamics setup displays antiresonant multiphoton transitions, as recently observed in a transmon qubit device. By including photon leaking, we explain the lineshape by a perturbative and a semiclassical analysis. We derive a bistable semiclassical quasienergy surface whose lowest quasienergy eigenstate is squeezed, allowing for a squeezing-dependent local effective temperature. We study the escape dynamics out of the metastable state and find signatures of dynamical tunneling, similar as for the quantum Duffing oscillator.Comment: submitted to PR

BCS theory of driven superconductivity

We study the impact of a time-dependent external driving of the lattice phonons in a minimal model of a BCS superconductor. Upon evaluating the driving-induced vertex corrections of the phonon-mediated electron-electron interaction, we show that parametric phonon driving can be used to elevate the critical temperature $T_c$, while a dipolar phonon drive has no effect. We provide simple analytic expressions for the enhancement factor of $T_c$. Furthermore, a mean-field analysis of a nonlinear phonon-phonon interaction also shows that phonon anharmonicities further amplify $T_c$. Our results hold universally for the large class of normal BCS superconductors

Strong coupling theory for tunneling and vibrational relaxation in driven bistable systems

A study of the dynamics of a tunneling particle in a driven bistable potential which is moderately-to-strongly coupled to a bath is presented. Upon restricting the system dynamics to the Hilbert space spanned by the M lowest energy eigenstates of the bare static potential, a set of coupled non-Markovian master equations for the diagonal elements of the reduced density matrix, within the discrete variale representation, is derived. The resulting dynamics is in good agreement with predictions of ab-initio real-time path integral simulations. Numerous results, analytical as well as numerical, for the quantum relaxation rate and for the asymptotic populations are presented. Our method is particularly convenient to investigate the case of shallow, time-dependent potential barriers and moderate-to-strong damping, where both a semi-classical and a Redfield-type approach are inappropriate.Comment: 37 pages, 23 figure

Quantum coherent biomolecular energy transfer with spatially correlated fluctuations

We show that the quantum coherent transfer of excitations between biomolecular chromophores is strongly influenced by spatial correlations of the environmental fluctuations. The latter are due either to propagating environmental modes or to local fluctuations with a finite localization length. A simple toy model of a single donor-acceptor pair with spatially separated chromophore sites allows to investigate the influence of these spatial correlations on the quantum coherent excitation transfer. The sound velocity of the solvent determines the wave lengths of the environmental modes, which, in turn, has to be compared to the spatial distance of the chromophore sites. When the wave length exceeds the distance between donor and acceptor site, we find strong suppression of decoherence. In addition, we consider two spatially separated donor-acceptor pairs under the influence of propagating environmental modes. Depending on their wave lengths fixed by the sound velocity of the solvent material, the spatial range of correlations may extend over typical interpair distances, which can lead to an increase of the decohering influence of the solvent. Surprisingly, this effect is counteracted by increasing temperature

Ultraslow quantum dynamics in a sub-Ohmic heat bath

We show that the low-frequency modes of a sub-Ohmic bosonic heat bath generate an effective dynamical asymmetry for an intrinsically symmetric quantum spin -1/2. An initially fully polarized spin first decays towards a quasiequilibrium determined by the dynamical asymmetry, thereby showing coherent damped oscillations on the (fast) time scale of the spin splitting. On top of this, the dynamical asymmetry itself decays on an ultraslow time scale and vanishes asymptotically since the global equilibrium phase is symmetric. We quantitatively study the nature of the initial fast decay to the quasiequilibrium and discuss the features of ultraslow dynamics of the quasiequilibrium itself. The dynamical asymmetry is more pronounced for smaller values of the sub-Ohmic exponent and for lower temperatures, which emphasizes the quantum many-body nature of the effect. The symmetry breaking is related to the dynamic crossover between coherent and overdamped relaxation of the spin polarization and is not connected to the localization quantum phase transition. In addition to this delocalized phase, we identify a novel phase which is characterized by damped coherent oscillations in the localized phase. This allows for a sketch of the zero-temperature phase diagram of the sub-Ohmic spin-boson model with four distinct phases.Comment: published version (minor changes), 8 pages, 5 figure

Dynamics of the spin-boson model with a structured environment

We investigate the dynamics of the spin-boson model when the spectral density of the boson bath shows a resonance at a characteristic frequency $\Omega$ but behaves Ohmically at small frequencies. The time evolution of an initial state is determined by making use of the mapping onto a system composed of a quantum mechanical two-state system (TSS) which is coupled to a harmonic oscillator (HO) with frequency $\Omega$. The HO itself is coupled to an Ohmic environment. The dynamics is calculated by employing the numerically exact quasiadiabatic path-integral propagator technique. We find significant new properties compared to the Ohmic spin-boson model. By reducing the TSS-HO system in the dressed states picture to a three-level system for the special case at resonance, we calculate the dephasing rates for the TSS analytically. Finally, we apply our model to experimentally realized superconducting flux qubits coupled to an underdamped dc-SQUID detector.Comment: 26 pages, 11 figures, Chemical Physics Special Issue on the Spin-Boson Problem, ed. by H. Grabert and A. Nitzan, in pres